A versatile experimental system for tracking ultrafast chemical reactions with X-ray free-electron lasers

Tetsuo Katayama; Shunsuke Nozawa; Yasufumi Umena; Sunghee Lee; Tadashi Togashi; Shigeki Owada; Makina Yabashi

doi:10.1063/1.5111795

A versatile experimental system for tracking ultrafast chemical reactions with X-ray free-electron lasers

Tetsuo Katayama, Shunsuke Nozawa, Yasufumi Umena, Sunghee Lee, Tadashi Togashi, Shigeki Owada, Makina Yabashi

Research Institute for Interdisciplinary Science

Research output: Contribution to journal › Article › peer-review

10 Citations (Scopus)

Abstract

An experimental system, SPINETT (SACLA Pump-probe INstrumEnt for Tracking Transient dynamics), dedicated for ultrafast pump-probe experiments using X-ray free-electron lasers has been developed. SPINETT consists of a chamber operated under 1 atm helium pressure, two Von Hamos spectrometers, and a large two-dimensional detector having a short work distance. This platform covers complementary X-ray techniques; one can perform time-resolved X-ray absorption spectroscopy, time-resolved X-ray emission spectroscopy, and time-resolved X-ray diffuse scattering. Two types of liquid injectors have been prepared for low-viscosity chemical solutions and for protein microcrystals embedded in a matrix. We performed a test experiment at SPring-8 Angstrom Compact free-electron LAser and demonstrated the capability of SPINETT to obtain the local electronic structure and geometrical information simultaneously.

Original language	English
Article number	054302
Journal	Structural Dynamics
Volume	6
Issue number	5
DOIs	https://doi.org/10.1063/1.5111795
Publication status	Published - Sept 1 2019

ASJC Scopus subject areas

Radiation
Instrumentation
Condensed Matter Physics
Spectroscopy

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title = "A versatile experimental system for tracking ultrafast chemical reactions with X-ray free-electron lasers",

abstract = "An experimental system, SPINETT (SACLA Pump-probe INstrumEnt for Tracking Transient dynamics), dedicated for ultrafast pump-probe experiments using X-ray free-electron lasers has been developed. SPINETT consists of a chamber operated under 1 atm helium pressure, two Von Hamos spectrometers, and a large two-dimensional detector having a short work distance. This platform covers complementary X-ray techniques; one can perform time-resolved X-ray absorption spectroscopy, time-resolved X-ray emission spectroscopy, and time-resolved X-ray diffuse scattering. Two types of liquid injectors have been prepared for low-viscosity chemical solutions and for protein microcrystals embedded in a matrix. We performed a test experiment at SPring-8 Angstrom Compact free-electron LAser and demonstrated the capability of SPINETT to obtain the local electronic structure and geometrical information simultaneously.",

author = "Tetsuo Katayama and Shunsuke Nozawa and Yasufumi Umena and Sunghee Lee and Tadashi Togashi and Shigeki Owada and Makina Yabashi",

note = "Funding Information: We greatly thank the staff of SACLA for their support and contribution. This research was performed with the approval of Japan Synchrotron Radiation Research Institute (JASRI; Proposal No. 2018B8062). JSPS KAKENHI Grant Nos. JP19H04407, JP19H05782, JP17H06438, and JP17H06141 supported this work. Publisher Copyright: {\textcopyright} 2019 Author(s).",

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doi = "10.1063/1.5111795",

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AU - Katayama, Tetsuo

AU - Nozawa, Shunsuke

AU - Umena, Yasufumi

AU - Lee, Sunghee

AU - Togashi, Tadashi

AU - Owada, Shigeki

AU - Yabashi, Makina

N1 - Funding Information: We greatly thank the staff of SACLA for their support and contribution. This research was performed with the approval of Japan Synchrotron Radiation Research Institute (JASRI; Proposal No. 2018B8062). JSPS KAKENHI Grant Nos. JP19H04407, JP19H05782, JP17H06438, and JP17H06141 supported this work. Publisher Copyright: © 2019 Author(s).

PY - 2019/9/1

Y1 - 2019/9/1

N2 - An experimental system, SPINETT (SACLA Pump-probe INstrumEnt for Tracking Transient dynamics), dedicated for ultrafast pump-probe experiments using X-ray free-electron lasers has been developed. SPINETT consists of a chamber operated under 1 atm helium pressure, two Von Hamos spectrometers, and a large two-dimensional detector having a short work distance. This platform covers complementary X-ray techniques; one can perform time-resolved X-ray absorption spectroscopy, time-resolved X-ray emission spectroscopy, and time-resolved X-ray diffuse scattering. Two types of liquid injectors have been prepared for low-viscosity chemical solutions and for protein microcrystals embedded in a matrix. We performed a test experiment at SPring-8 Angstrom Compact free-electron LAser and demonstrated the capability of SPINETT to obtain the local electronic structure and geometrical information simultaneously.

AB - An experimental system, SPINETT (SACLA Pump-probe INstrumEnt for Tracking Transient dynamics), dedicated for ultrafast pump-probe experiments using X-ray free-electron lasers has been developed. SPINETT consists of a chamber operated under 1 atm helium pressure, two Von Hamos spectrometers, and a large two-dimensional detector having a short work distance. This platform covers complementary X-ray techniques; one can perform time-resolved X-ray absorption spectroscopy, time-resolved X-ray emission spectroscopy, and time-resolved X-ray diffuse scattering. Two types of liquid injectors have been prepared for low-viscosity chemical solutions and for protein microcrystals embedded in a matrix. We performed a test experiment at SPring-8 Angstrom Compact free-electron LAser and demonstrated the capability of SPINETT to obtain the local electronic structure and geometrical information simultaneously.

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A versatile experimental system for tracking ultrafast chemical reactions with X-ray free-electron lasers

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