Catalytic sites of mesoporous silica in degradation of polyethylene

A. Satsuma; T. Ebigase; Y. Inaki; H. Yoshida; S. Kobayashi; M. A. Uddin; Y. Sakata; T. Hattori

doi:10.1016/S0167-2991(01)81607-4

Catalytic sites of mesoporous silica in degradation of polyethylene

A. Satsuma, T. Ebigase, Y. Inaki, H. Yoshida, S. Kobayashi, M. A. Uddin, Y. Sakata, T. Hattori

Institute for Global Human Resource Development

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

7 Citations (Scopus)

Abstract

Catalytic sites of mesoporous silica catalysts in degradation of polyethylene were studied using characterizations by adsorption of NH₃ and isohexane cracking. Siliceous materials showed a high liquid yield close to that of non-catalytic run, and degradation rate was improved by incorporation of aluminum. Mesoporous silica containing impurity level of aluminum showed high activity, same with H-MFI and SiO₂-A1₂0₃ with similar A1 content. The initial rate of degradation was dependent on the aluminum content and structure of mesoporous silica catalysts. FSM-16 exhibited exceptionally higher activity, which may be due to the presence of radical type catalytic sites on FSM-16. This is an abstract of a paper presented at the 13^th International Zeolite Conference (Montpellier, France 7/8-13/2001).

Original language	English
Title of host publication	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001
Publisher	Elsevier Inc.
Pages	277
Number of pages	1
Volume	135
ISBN (Print)	9780444502384
DOIs	https://doi.org/10.1016/S0167-2991(01)81607-4
Publication status	Published - 2001
Event	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001 - Montpellier, France Duration: Jun 8 2001 → Jun 13 2001

Other

Other	Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001
Country/Territory	France
City	Montpellier
Period	6/8/01 → 6/13/01

ASJC Scopus subject areas

Catalysis
Condensed Matter Physics
Surfaces, Coatings and Films
Physical and Theoretical Chemistry
Materials Chemistry

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10.1016/S0167-2991(01)81607-4

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Satsuma, A., Ebigase, T., Inaki, Y., Yoshida, H., Kobayashi, S., Uddin, M. A., Sakata, Y., & Hattori, T. (2001). Catalytic sites of mesoporous silica in degradation of polyethylene. In Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001 (Vol. 135, pp. 277). Elsevier Inc.. https://doi.org/10.1016/S0167-2991(01)81607-4

Satsuma, A, Ebigase, T, Inaki, Y, Yoshida, H, Kobayashi, S, Uddin, MA, Sakata, Y & Hattori, T 2001, Catalytic sites of mesoporous silica in degradation of polyethylene. in Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001. vol. 135, Elsevier Inc., pp. 277, Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001, Montpellier, France, 6/8/01. https://doi.org/10.1016/S0167-2991(01)81607-4

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abstract = "Catalytic sites of mesoporous silica catalysts in degradation of polyethylene were studied using characterizations by adsorption of NH3 and isohexane cracking. Siliceous materials showed a high liquid yield close to that of non-catalytic run, and degradation rate was improved by incorporation of aluminum. Mesoporous silica containing impurity level of aluminum showed high activity, same with H-MFI and SiO2-A1203 with similar A1 content. The initial rate of degradation was dependent on the aluminum content and structure of mesoporous silica catalysts. FSM-16 exhibited exceptionally higher activity, which may be due to the presence of radical type catalytic sites on FSM-16. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).",

author = "A. Satsuma and T. Ebigase and Y. Inaki and H. Yoshida and S. Kobayashi and Uddin, {M. A.} and Y. Sakata and T. Hattori",

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T1 - Catalytic sites of mesoporous silica in degradation of polyethylene

AU - Satsuma, A.

AU - Ebigase, T.

AU - Inaki, Y.

AU - Yoshida, H.

AU - Kobayashi, S.

AU - Uddin, M. A.

AU - Sakata, Y.

AU - Hattori, T.

PY - 2001

Y1 - 2001

N2 - Catalytic sites of mesoporous silica catalysts in degradation of polyethylene were studied using characterizations by adsorption of NH3 and isohexane cracking. Siliceous materials showed a high liquid yield close to that of non-catalytic run, and degradation rate was improved by incorporation of aluminum. Mesoporous silica containing impurity level of aluminum showed high activity, same with H-MFI and SiO2-A1203 with similar A1 content. The initial rate of degradation was dependent on the aluminum content and structure of mesoporous silica catalysts. FSM-16 exhibited exceptionally higher activity, which may be due to the presence of radical type catalytic sites on FSM-16. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).

AB - Catalytic sites of mesoporous silica catalysts in degradation of polyethylene were studied using characterizations by adsorption of NH3 and isohexane cracking. Siliceous materials showed a high liquid yield close to that of non-catalytic run, and degradation rate was improved by incorporation of aluminum. Mesoporous silica containing impurity level of aluminum showed high activity, same with H-MFI and SiO2-A1203 with similar A1 content. The initial rate of degradation was dependent on the aluminum content and structure of mesoporous silica catalysts. FSM-16 exhibited exceptionally higher activity, which may be due to the presence of radical type catalytic sites on FSM-16. This is an abstract of a paper presented at the 13th International Zeolite Conference (Montpellier, France 7/8-13/2001).

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SN - 9780444502384

VL - 135

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BT - Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001

PB - Elsevier Inc.

T2 - Zeolites and Mesoporous Materials at the dawn of the 21st century, Proceedings of the 13 International Zeolite Conference, 2001

Y2 - 8 June 2001 through 13 June 2001

ER -

Catalytic sites of mesoporous silica in degradation of polyethylene

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