TY - JOUR
T1 - Charge-neutral fermions and magnetic field-driven instability in insulating YbIr3Si7
AU - Sato, Y.
AU - Suetsugu, S.
AU - Tominaga, T.
AU - Kasahara, Y.
AU - Kasahara, S.
AU - Kobayashi, T.
AU - Kitagawa, Shunsaku
AU - Ishida, K.
AU - Peters, R.
AU - Shibauchi, T.
AU - Nevidomskyy, A. H.
AU - Qian, L.
AU - Morosan, E.
AU - Matsuda, Y.
N1 - Funding Information:
A.H.N. and E.M. acknowledge fruitful discussions with Chris Hooley. Y.M. acknowledges discussion with H. Kontani, Lu Li, and J. Singleton. L.Q., and E.M. acknowledge support from the U.S. Department of Energy for Grant No. DE-SC0019503. A.H.N. was supported by the National Science Foundation grant No. DMR-1917511 and the Robert A. Welch Foundation grant C-1818. This work is supported by Grants-in-Aid for Scientific Research (KAKENHI) (Nos. JP15H02106, JP18H01177, JP18H01178, JP18H01180, JP18H05227, JP19H00649, JP20H02600, JP18K03511, and JP20H05159) and on Innovative Areas “Quantum Liquid Crystals” (No. JP19H05824) from Japan Society for the Promotion of Science (JSPS), and JST CREST (JP-MJCR19T5).
Publisher Copyright:
© 2022, The Author(s).
PY - 2022/12
Y1 - 2022/12
N2 - Kondo lattice materials, where localized magnetic moments couple to itinerant electrons, provide a very rich backdrop for strong electron correlations. They are known to realize many exotic phenomena, with a dramatic example being recent observations of quantum oscillations and metallic thermal conduction in insulators, implying the emergence of enigmatic charge-neutral fermions. Here, we show that thermal conductivity and specific heat measurements in insulating YbIr3Si7 reveal emergent neutral excitations, whose properties are sensitively changed by a field-driven transition between two antiferromagnetic phases. In the low-field phase, a significant violation of the Wiedemann-Franz law demonstrates that YbIr3Si7 is a charge insulator but a thermal metal. In the high-field phase, thermal conductivity exhibits a sharp drop below 300 mK, indicating a transition from a thermal metal into an insulator/semimetal driven by the magnetic transition. These results suggest that spin degrees of freedom directly couple to the neutral fermions, whose emergent Fermi surface undergoes a field-driven instability at low temperatures.
AB - Kondo lattice materials, where localized magnetic moments couple to itinerant electrons, provide a very rich backdrop for strong electron correlations. They are known to realize many exotic phenomena, with a dramatic example being recent observations of quantum oscillations and metallic thermal conduction in insulators, implying the emergence of enigmatic charge-neutral fermions. Here, we show that thermal conductivity and specific heat measurements in insulating YbIr3Si7 reveal emergent neutral excitations, whose properties are sensitively changed by a field-driven transition between two antiferromagnetic phases. In the low-field phase, a significant violation of the Wiedemann-Franz law demonstrates that YbIr3Si7 is a charge insulator but a thermal metal. In the high-field phase, thermal conductivity exhibits a sharp drop below 300 mK, indicating a transition from a thermal metal into an insulator/semimetal driven by the magnetic transition. These results suggest that spin degrees of freedom directly couple to the neutral fermions, whose emergent Fermi surface undergoes a field-driven instability at low temperatures.
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U2 - 10.1038/s41467-021-27541-9
DO - 10.1038/s41467-021-27541-9
M3 - Article
C2 - 35046390
AN - SCOPUS:85123047246
SN - 2041-1723
VL - 13
JO - Nature communications
JF - Nature communications
IS - 1
M1 - 394
ER -