TY - JOUR
T1 - Experimental study of thermal conductivity at high pressures
T2 - Implications for the deep Earth's interior
AU - Goncharov, Alexander F.
AU - Lobanov, Sergey S.
AU - Tan, Xiaojing
AU - Hohensee, Gregory T.
AU - Cahill, David G.
AU - Lin, Jung Fu
AU - Thomas, Sylvia Monique
AU - Okuchi, Takuo
AU - Tomioka, Naotaka
N1 - Funding Information:
We thank Brent Grocholski from Smithsonian Institution for providing the ferropericlase sample. We acknowledge support from the NSF EAR , NSF EAR/IF , Army Research Office , DARPA and EFREE, a BES-EFRC center at Carnegie . S.S.L. was partly supported by the Ministry of Education and Science of Russian Federation (Grant No. 14.B25.31.0032 ). G.T.H. and D.G.C. acknowledge support from the Carnegie-DOE Alliance Center (CDAC) . S.M.T. acknowledges support from NSF EAR Grants 1215957 and 1417274 . J.F.L. acknowledges financial support from NSF Earth Sciences ( EAR-0838221 and EAR-1446946 ), Deep Carbon Observatory, and the Visiting Professorship Program at the Institute for the Study of the Earth’s Interior of the Okayama University at Misasa .
Publisher Copyright:
© 2015 Elsevier B.V.
PY - 2014/8/25
Y1 - 2014/8/25
N2 - Lattice thermal conductivity of ferropericlase and radiative thermal conductivity of iron bearing magnesium silicate perovskite (bridgmanite) - the major mineral of Earth's lower mantle- have been measured at room temperature up to 30 and 46GPa, respectively, using time-domain thermoreflectance and optical spectroscopy techniques in diamond anvil cells. The results provide new constraints for the pressure dependencies of the thermal conductivities of Fe bearing minerals. The lattice thermal conductivity of ferropericlase Mg0.9Fe0.1O is 5.7(6)W/(m*K) at ambient conditions, which is almost 10 times smaller than that of pure MgO; however, it increases with pressure much faster (6.1(7)%/GPa vs 3.6(1)%/GPa). The radiative conductivity of a Mg0.94Fe0.06SiO3 bridgmanite single crystal agrees with previously determined values for powder samples at ambient pressure; it is almost pressure-independent in the investigated pressure range. Our results confirm the reduced radiative conductivity scenario for the Earth's lower mantle, while the assessment of the heat flow through the core-mantle boundary still requires in situ measurements at the relevant pressure-temperature conditions.
AB - Lattice thermal conductivity of ferropericlase and radiative thermal conductivity of iron bearing magnesium silicate perovskite (bridgmanite) - the major mineral of Earth's lower mantle- have been measured at room temperature up to 30 and 46GPa, respectively, using time-domain thermoreflectance and optical spectroscopy techniques in diamond anvil cells. The results provide new constraints for the pressure dependencies of the thermal conductivities of Fe bearing minerals. The lattice thermal conductivity of ferropericlase Mg0.9Fe0.1O is 5.7(6)W/(m*K) at ambient conditions, which is almost 10 times smaller than that of pure MgO; however, it increases with pressure much faster (6.1(7)%/GPa vs 3.6(1)%/GPa). The radiative conductivity of a Mg0.94Fe0.06SiO3 bridgmanite single crystal agrees with previously determined values for powder samples at ambient pressure; it is almost pressure-independent in the investigated pressure range. Our results confirm the reduced radiative conductivity scenario for the Earth's lower mantle, while the assessment of the heat flow through the core-mantle boundary still requires in situ measurements at the relevant pressure-temperature conditions.
KW - Bridgmanite
KW - Deep Earth's minerals
KW - Ferropericlase
KW - High pressure
KW - Lattice thermal conductivity
KW - Lower mantle
KW - Optical properties
KW - Radiative conductivity
KW - Thermal conductivity
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U2 - 10.1016/j.pepi.2015.02.004
DO - 10.1016/j.pepi.2015.02.004
M3 - Article
AN - SCOPUS:84945484973
SN - 0031-9201
VL - 247
SP - 11
EP - 16
JO - Physics of the Earth and Planetary Interiors
JF - Physics of the Earth and Planetary Interiors
ER -