Chiral pyrophosphoric acid catalysts for the para-selective and enantioselective aza-friedel-crafts reaction of phenols

Haruka Okamoto, Kohei Toh, Takuya Mochizuki, Hidefumi Nakatsuji, Akira Sakakura, Manabu Hatano, Kazuaki Ishihara

研究成果査読

9 被引用数 (Scopus)

抄録

Chiral BINOL-derived pyrophosphoric acid catalysts were developed and used for the regio- and enantioselective aza-Friedel-Crafts reaction of phenols with aldimines. ortho/para-Directing phenols could react at the para-position selectively with moderate to good enantioselectivities. Moreover, the gram-scale transformation of a product into the key intermediate for the antifungal agent (R)-bifonazole was demonstrated.

本文言語English
ページ(範囲)4577-4590
ページ数14
ジャーナルSynthesis (Germany)
50
23
DOI
出版ステータスPublished - 2018

ASJC Scopus subject areas

  • 触媒
  • 有機化学

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