Isokinetic approach in logarithmic mean-force dynamics for on-the-fly free energy reconstruction

Tetsuya Morishita, Takenobu Nakamura, Wataru Shinoda, Atsushi M. Ito

研究成果査読

4 被引用数 (Scopus)

抄録

Logarithmic mean-force dynamics (LogMFD) is one of free energy calculation methods that utilize fictitious dynamical variables for efficient conformational sampling. In this study, we extend the LogMFD method to incorporate the isokinetic dynamics for the fictitious dynamical variables. The isokinetic LogMFD approach requires no additional parameter for thermostatting and it obviates the issue associated with the dynamics of the thermostat variable in Nosé-Hoover type thermostats. These virtues therefore make it easier to set up and undertake LogMFD calculations. The validity of the isokinetic algorithm introduced in LogMFD is examined by a benchmark system of alanine dipeptide in explicit water.

本文言語English
ページ(範囲)633-640
ページ数8
ジャーナルChemical Physics Letters
706
DOI
出版ステータスPublished - 8月 16 2018
外部発表はい

ASJC Scopus subject areas

  • 物理学および天文学(全般)
  • 物理化学および理論化学

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